With the AW4 on the highway you would still be in a low comfortable cruising RPM at 3.54. I think the Eagle moves around a little better at around 2250 RPM on the highway. Below 1900 RPM is best left to Spirits, Gremlins, and Pacers.
Looking at the stock Cherokee, which took a lot from the Eagle, they were set up with 3.54 for the AW4 and 3.07 for the T5, and I had no problem getting 20 MPG in one with the AW4 so long as I kept it under 60, but the Eagle should fare better at 65-70 because it's not a big square brick. The limit on the Cherokee and Wrangler is really the aerodynamics.
The big 235/75 tires will hurt city fuel economy, it's more mass on the outside of a larger diameter wheel and the engine has to break the inertia of them each time you start, and if you want to stick with them I'd lean more toward the 3.54. If you were planning on the smaller sizes then the 3.31 would make more sense.
Unfortunately, you are going to be hunting for 3.31 if you go that way. They were only offered in '81 on Eagles and are rare in Jeeps.
I've been using
http://www.grimmjeeper.com/gears.html, it's nice to compare, but the "copy" buttons seem backward to me. It's got most common transmissions in it.